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Optical studies of physical properti...

Columbia University.

Optical studies of physical properties of nano-structures.

紀錄類型:	書目-電子資源 : 單行本
正題名/作者:	Optical studies of physical properties of nano-structures./
作者:	Song, Daohua.
面頁冊數:	141 p.
附註:	Source: Dissertation Abstracts International, Volume: 68-10, Section: B, page: 6722.
Contained By:	Dissertation Abstracts International68-10B.
標題:	Physics, Condensed Matter. -
電子資源:	Download PDF (下載PDF全文)
ISBN:	9780549269571

Optical studies of physical properties of nano-structures.
Song, Daohua.

Optical studies of physical properties of nano-structures. - 141 p.

Source: Dissertation Abstracts International, Volume: 68-10, Section: B, page: 6722.

Thesis (Ph.D.)--Columbia University, 2007.

This thesis is divided into two parts. The first part of this dissertation describes the motivation and background, theory and experimental methods of using linear and nonlinear optical techniques to probe the phase transitions of ferroelectric materials. In the second part, femtosecond time-resolved spectroscopy is applied to monitor the real-time response of the electronic structure and lattice vibrations to external perturbation.

ISBN: 9780549269571Subjects--Topical Terms:

1000005552
Physics, Condensed Matter.

Optical studies of physical properties of nano-structures.
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245 1 0 $a Optical studies of physical properties of nano-structures.
300 $a 141 p.
500 $a Source: Dissertation Abstracts International, Volume: 68-10, Section: B, page: 6722.
500 $a Adviser: Tony F. Heinz.
502 $a Thesis (Ph.D.)--Columbia University, 2007.
520 $a This thesis is divided into two parts. The first part of this dissertation describes the motivation and background, theory and experimental methods of using linear and nonlinear optical techniques to probe the phase transitions of ferroelectric materials. In the second part, femtosecond time-resolved spectroscopy is applied to monitor the real-time response of the electronic structure and lattice vibrations to external perturbation.
520 $a With respect to ferroelectric materials, our research is motivated by a desire to understand the finite size effects of ferroelectricity in the nanometer size range. For this purpose we applied the optical second-harmonic generation (SHG) technique, a method which has already been proved to be a powerful probe of bulk ferroelectricities. Here for the first time, we demonstrate SHG as a tool to study finite size effects, with sensitivity down to an individual nanoscale object. Experimentally, we examined BaTi2O5 nanowires as a model system. Compared to the bulk, a much lower phase transition temperature is observed for single BaTi2O 5 nanowires with diameter around 50 nm. Explanations and future work are proposed.
520 $a The system of single-walled carbon nanotubes (SWNTs) has attracted much recent attention both as a model one-dimensional material and for its potential for diverse applications. In this thesis we present results of two fundamental studies of the properties of SWNTs probed by ultrafast laser pulses.
520 $a The first investigation is a measurement of the optical Stark effect (OSE) in SWNTs, that is, the shift in the optical transition energy induced by strong off-resonance light fields. This effect is explored experimentally using a femtosecond infrared pulse to induce the OSE and a femtosecond pulse resonant with an excitonic transition to probe the response. We observe a significant and instantaneous blue shift of the transition. The strength of the OSE is attributed to the enhanced Coulomb interactions present in these one-dimensional materials.
520 $a The second investigation uses time-resolved anti-Stokes Raman scattering for a direct determination of the lifetime of the zone-center (G mode) optical phonons in semiconducting SWNTs. For (6,5) nanotubes, a lifetime of just over 1 ps is obtained. In addition to its intrinsic interest as a measure of phonon-phonon coupling, this lifetime is important in assessing the role of non-equilibrium phonon populations in high-field transport phenomena.
590 $a School code: 0054.
650 4 $a Physics, Condensed Matter. $3 1000005552
650 4 $a Physics, Optics. $3 1000005523
690 $a 0611
690 $a 0752
710 2 $a Columbia University. $3 1000005501
773 0 $t Dissertation Abstracts International $g 68-10B.
790 1 0 $a Heinz, Tony F., $e advisor
790 $a 0054
791 $a Ph.D.
792 $a 2007
856 4 0 $u http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3285169 $z Download PDF (下載PDF全文)